126 51 1430 3 3101 document 1430 Dataset_for_hot_electron_dynamics.xlsx application/vnd.openxmlformats-officedocument.spreadsheetml.sheet 20880afd379d261fc251131a7343da1d MD5 911437 2015-08-03 15:47:03 https://researchdata.bath.ac.uk/126/1/Dataset_for_hot_electron_dynamics.xlsx 126 1 1 application/vnd.openxmlformats-officedocument.spreadsheetml.sheet other Complete data set for publication en public cc_by

Dataset_for_hot_electron_dynamics.xlsx

data 1431 3 3115 document 1431 Lock_local_toluene_room_temp.csv text/plain e3d9824b5c656eb07540815235a9c2c6 MD5 6253 2015-08-04 10:04:13 https://researchdata.bath.ac.uk/126/2/Lock_local_toluene_room_temp.csv 126 2 2 text/plain other Room temperature data for local manipulation of toluene molecules. en public cc_by

Lock_local_toluene_room_temp.csv

data 1432 3 3117 document 1432 Lock_nonlocal_benzene_room_temp.csv text/plain e5cb8156cfb5a35a1f6f21713f5377ce MD5 386896 2015-08-04 10:04:25 https://researchdata.bath.ac.uk/126/3/Lock_nonlocal_benzene_room_temp.csv 126 3 3 text/plain other Room temperature data for nonlocal manipulation of benzene molecules. en public cc_by

Lock_nonlocal_benzene_room_temp.csv

data 1433 3 3119 document 1433 Lock_nonlocal_chlorobenzene_room_temp.csv text/plain 7b946719b126ec5d73bb9473a49baaef MD5 51588 2015-08-04 10:04:30 https://researchdata.bath.ac.uk/126/4/Lock_nonlocal_chlorobenzene_room_temp.csv 126 4 4 text/plain other Room temperature data for local manipulation of chlorobenzene molecules. en public cc_by

Lock_nonlocal_chlorobenzene_room_temp.csv

data 1434 3 3121 document 1434 Lock_nonlocal_chlorobenzene_variable_temp.csv text/plain 77e9588b37835ab0be1cd8833a173aa8 MD5 7232 2015-08-04 10:04:32 https://researchdata.bath.ac.uk/126/5/Lock_nonlocal_chlorobenzene_variable_temp.csv 126 5 5 text/plain other Variable temperature data for nonlocal manipulation of chlorobenzene molecules. en public cc_by

Lock_nonlocal_chlorobenzene_variable_temp.csv

data 1435 3 3123 document 1435 Lock_nonlocal_toluene_room_temp.csv text/plain e14cd20bec7b03002d5ab812eb7d89c6 MD5 318346 2015-08-04 10:04:35 https://researchdata.bath.ac.uk/126/6/Lock_nonlocal_toluene_room_temp.csv 126 6 6 text/plain other Room temperature data for nonlocal manipulation of toluene molecules. en public cc_by

Lock_nonlocal_toluene_room_temp.csv

data archive 3089 disk0/00/00/01/26 2015-09-23 11:49:16 2024-07-15 10:57:50 2015-09-23 11:49:16 data_collection show Lock Duncan d.lock@bath.ac.uk University of Bath FALSE Rusimova Kristina k.r.rusimova@bath.ac.uk 0000-0002-3679-9948 University of Bath FALSE Pan Tianluo 0000-0002-9268-9567 University of Birmingham FALSE Palmer Richard r.e.palmer@bham.ac.uk University of Birmingham FALSE Sloan Peter p.sloan@bath.ac.uk 0000-0002-0810-8468 University of Bath TRUE CJ0020 KF0010 dept_physics The dynamics of hot electrons are central to understanding the properties of many electronic devices. But their ultra-short lifetime, typically 100 fs or less, and hence their corresponding transport length-scale of a few nanometers severely constrains real space investigations. Here we report variable temperature and voltage measurements of the nonlocal manipulation of adsorbed molecules on the Si(111)-7x7 surface in the scanning tunnelling microscope. The range of the nonlocal effect increases with temperature and, at constant temperature, is invariant over a wide range of electron energies. The measurements probe, in real space, the underlying hot electron dynamics on the 10 nm scale and are well described by a two-dimensional diffusive model with a single decay channel, consistent with 2PPE measurements of the real time dynamics. 2015 University of Bath public RightsHolder University of Bath Engineering and Physical Sciences Research Council https://doi.org/10.13039/501100000266 EP/K00137X/1 Breaking the Single Atom Limit in Atomic Manipulation Please see main paper methods section. For radial distributions we present the raw N/N0 and thermally corrected data as well, again see methods section for details. https://doi.org/10.1038/ncomms9365 en 1 10.15125/BATH-00126 https://doi.org/10.1038/ncomms9365 pub open All data files available under a CC-BY 4.0 licence.