This dataset contains scripts and data supporting the following following thesis: Pollet, M. (2025). Rapid structural analysis of prefabricated thin concrete shells using deep learning (Thesis). University of Bath. Concrete thin-shells are materially efficient structures, which can be used to reduce the environmental impact of concrete structures. However, geometric imperfections, which may occur during production can negatively impact their structural behaviour. While this impact can be assessed through Finite Element Analysis (FEA), a faster analysis method, such as surrogate modelling, could benefit concrete shell manufacturers. This dataset contains deep learning models – Multilayer Perceptrons, and Convolutional Neural Networks – that have been trained to predict the buckling factor and stress fields of geometrically imperfect concrete thin-shells of various shapes under design loads. It also contains the Python scripts that were used to train these models and assess their performance. Running these scripts necessitates the associated ConcreteShellFEA dataset to be downloaded. Further details about this data can be found in the related thesis.