Data for paper: Initiating and imaging the coherent surface dynamics of charge carriers in real space

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http://eprints.org/relation/isVersionOf https://researchdata.bath.ac.uk/id/document/4351 http://eprints.org/relation/isVolatileVersionOf https://researchdata.bath.ac.uk/id/document/4351 http://eprints.org/relation/isIndexCodesVersionOf https://researchdata.bath.ac.uk/id/document/4351 archive 3089 disk0/00/00/02/30 2016-09-29 09:19:19 2024-09-19 11:22:12 2016-09-29 09:19:19 data_collection show Sloan Peter P.Sloan@bath.ac.uk 0000-0002-0810-8468 University of Bath TRUE Rusimova Kristina K.R.Rusimova@bath.ac.uk 0000-0002-3679-9948 University of Bath FALSE Bannister Nicola N.Bannister@bath.ac.uk University of Bath FALSE Harrison Patrick 0000-0001-9798-8710 University of Birmingham FALSE Crampin Simon S.Crampin@bath.ac.uk 0000-0002-1152-231X University of Bath FALSE Palmer Richard r.e.palmer@bham.ac.uk University of Birmingham FALSE Lock Duncan D.Lock@bath.ac.uk University of Bath FALSE Data for paper: Initiating and imaging the coherent surface dynamics of charge carriers in real space CJ0020 KF0010 dept_physics SJB Custom Low Temperature STM The tip of a scanning tunnelling microscope is an atomic-scale source of electrons and holes. As the injected charge spreads out it can induce adsorbed molecules to react. By comparing large-scale `before' and `after' images of an adsorbate covered surface, the spatial extent of the nonlocal manipulation is revealed. Here we measure the nonlocal manipulation of toluene molecules on the Si(111)-7x7 surface at room temperature. Both the range and probability of nonlocal manipulation have a voltage dependence. A region within 5 to 15 nm of the injection site shows a marked reduction in manipulation. We propose that this region marks the extent of the initial coherent (i.e., ballistic) time-dependent evolution of the injected charge carrier. Using scanning tunnelling spectroscopy, we develop a model of this time-dependent expansion of the initially localized hole wavepacket within a particular surface state and deduce a quantum coherence (ballistic) lifetime of about 10 fs. 2016-07-27 University of Bath public RightsHolder University of Bath Engineering and Physical Sciences Research Council https://doi.org/10.13039/501100000266 EP/K00137X/1 Breaking the Single Atom Limit in Atomic Manipulation Please see main paper methods section. For radial distributions we present the thermally corrected N/N0 data, again see methods section for details. https://doi.org/10.1038/ncomms12839 2014-09-20 2015-09-01 2012-01-01 2016-01-01 en 1 10.15125/BATH-00230 https://doi.org/10.1016/B978-0-08-096355-6.00005-2 pub https://doi.org/10.1103/PhysRevLett.105.048301 pub https://doi.org/10.1038/ncomms9365 pub https://doi.org/10.1088/0953-8984/27/5/054003 pub https://doi.org/10.1002/tcr.201402021 pub https://doi.org/10.1038/ncomms12839 pub