Dataset for "Interactions of Choline and Geranate (CAGE) Deep Eutectic Solvents with Lipid Bilayers" Note: Beamline data from the FIGARO specular NR instrument at The I.L.L., France can be found here: DOI:10.5291/ILL-DATA.9-13-927 Contents: Main Article: Figure3 (DLS): Raw DLS traces for 100 mM aqueous CAGE and CAOT suspensions in 1:1 and 1:2 ratios. Figure4: (QCM-D; 1-2 materials) Raw and relative QCM-D traces for response of SLBs (5 MHz SiO2) and SVLs (10 MHz Au) to 1:2 CAGE or CAOT. Figure5: (QCM-D); 1-1 materials) Raw and relative QCM-D traces for response of SLBs(5 MHz SiO2) and SVLs (10 MHz Au) to 1:1 CAGE or CAOT. Supporting Information: Figure S1 (DLS, SAXS) Figure S1a (DLS): Raw DLS traces for DMPC SUV suspension (5 mg/ml) in PBS. Figure S1b (SAXS): Raw SAXS data for SUV suspensions and PBS. Including background subtracted data and data converted to per angstrom. Figure S2 (QCM-D) Raw and relative QCM-D traces for deposition of SVL on Au (10 MHz) and SLB on SiO2 (5 MHz). Figure S4 (QCM-D) Raw and relative QCM-D traces (10 MHz Au) for deposition of SVL followed by response to 0.3 and 10.0 mM aqueous CAGE suspensions. Figure S5 (1H NMR) 1H NMR spectrum for CAOT from hCh-hOT in D2O (25 oC) Figure S6 (1H NMR) 1H NMR spectrum for CAOT from hCh-dOT in D2O (25oC) Figure S18 (DFT Modelling) Log files from DFT modelling, visualisations and averaging of molecular volumes.