Atomically resolved real-space imaging of hot electron dynamics
The dynamics of hot electrons are central to understanding the properties of many electronic devices. But their ultra-short lifetime, typically 100 fs or less, and hence their corresponding transport length-scale of a few nanometers severely constrains real space investigations. Here we report variable temperature and voltage measurements of the nonlocal manipulation of adsorbed molecules on the Si(111)-7x7 surface in the scanning tunnelling microscope. The range of the nonlocal effect increases with temperature and, at constant temperature, is invariant over a wide range of electron energies. The measurements probe, in real space, the underlying hot electron dynamics on the 10 nm scale and are well described by a two-dimensional diffusive model with a single decay channel, consistent with 2PPE measurements of the real time dynamics.
Cite this dataset as:
Lock, D.,
Rusimova, K.,
Pan, T.,
Palmer, R.,
Sloan, P.,
2015.
Atomically resolved real-space imaging of hot electron dynamics.
Bath: University of Bath Research Data Archive.
Available from: https://doi.org/10.15125/BATH-00126.
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Data
Dataset_for … electron_dynamics.xlsx
application/vnd.openxmlformats-officedocument.spreadsheetml.sheet (911kB)
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Complete data set for publication
Lock_local_toluene_room_temp.csv
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Room temperature data for local manipulation of toluene molecules.
Lock_nonlocal … room_temp.csv
text/plain (386kB)
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Room temperature data for nonlocal manipulation of benzene molecules.
Lock_nonlocal … room_temp.csv
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Room temperature data for local manipulation of chlorobenzene molecules.
Lock_nonlocal … variable_temp.csv
text/plain (7kB)
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Variable temperature data for nonlocal manipulation of chlorobenzene molecules.
Lock_nonlocal … room_temp.csv
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Room temperature data for nonlocal manipulation of toluene molecules.
All data files available under a CC-BY 4.0 licence.
Creators
Duncan Lock
University of Bath
Kristina Rusimova
University of Bath
Tianluo Pan
University of Birmingham
Richard Palmer
University of Birmingham
Peter Sloan
University of Bath
Contributors
University of Bath
Rights Holder
Documentation
Data collection method:
Please see main paper methods section. For radial distributions we present the raw N/N0 and thermally corrected data as well, again see methods section for details.
Methodology link:
Lock, D., Rusimova, K. R., Pan, T. L., Palmer, R. E., and Sloan, P. A., 2015. Atomically resolved real-space imaging of hot electron dynamics. Nature Communications, 6(1). Available from: https://doi.org/10.1038/ncomms9365.
Funders
Engineering and Physical Sciences Research Council
https://doi.org/10.13039/501100000266
Breaking the Single Atom Limit in Atomic Manipulation
EP/K00137X/1
Publication details
Publication date: 2015
by: University of Bath
Version: 1
DOI: https://doi.org/10.15125/BATH-00126
URL for this record: https://researchdata.bath.ac.uk/id/eprint/126
Related papers and books
Lock, D., Rusimova, K. R., Pan, T. L., Palmer, R. E., and Sloan, P. A., 2015. Atomically resolved real-space imaging of hot electron dynamics. Nature Communications, 6(1). Available from: https://doi.org/10.1038/ncomms9365.
Contact information
Please contact the Research Data Service in the first instance for all matters concerning this item.
Contact person: Peter Sloan
Faculty of Science
Physics
