Data set for "Doubly-resonant enhancement of Second Harmonic Generation from a WS2 nanomesh polymorph with a modified energy landscape"

WS2 is an example of a transition metal dichalcogenide, and a highly promising 2D material for nonlinear optics. This dataset contains plots of multiphoton emission spectra and coordinates of second harmonic generation (SHG) hotspots of WS2 polymorphs and thin films formed into a nanomesh, that is, a tridimensional webbed network of densely-packed stacks (of 1–5 layers) of twisted and/or fused 2D nanosheets. The locations of the emission hotspots were determined by illumination at 1225, 1050, and 850 nm incident wavelengths.

Subjects:
Materials sciences
Optics, photonics and lasers

Cite this dataset as:
Murphy, A., Liu, Z., Gorbach, A., Ilie, A., Valev, V., 2021. Data set for "Doubly-resonant enhancement of Second Harmonic Generation from a WS2 nanomesh polymorph with a modified energy landscape". Bath: University of Bath Research Data Archive. Available from: https://doi.org/10.15125/BATH-00989.

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Data

Pixel Intensity … Sample 6.opju
application/octet-stream (81kB)
Creative Commons: Attribution 4.0

Plot of pixel intensity versus wavelength (Figure 3 in the paper)

Second attempt … coordinates.xlsx
application/vnd.openxmlformats-officedocument.spreadsheetml.sheet (9kB)
Creative Commons: Attribution 4.0

Second harmonic generation (SHG) hotspot coordinates

Creators

Alexander Murphy
Data Collector
University of Bath

Zichen Liu
Researcher
University of Bath

Andriy Gorbach
Researcher
University of Bath

Adelina Ilie
Researcher
University of Bath

Ventsislav Valev
Supervisor
University of Bath

Contributors

University of Bath
Rights Holder

Documentation

Data collection method:

Multiphoton imaging: Samples were illuminated from 850 to 1300 nm in incrememnts of 25 nm with a constant average power of 0.5 mW. Images of the emission from 425 to 650 in 32 steps were taken.

Data processing and preparation activities:

An in house script was used to take the resulting images, convert them to greyscale and averaging the pic intensity in the area specified using the coordinates chosen or the whole of the image. The resultant data was then plotted.

Technical details and requirements:

Zen Blue was used to obtain the data and Zen Black to convert the .czi to .jif files. A python script was then used and results in a .csv file. Origin was then used to plot the data.

Additional information:

Hotspot coordinates are provided in MS Excel format. The plot of pixel intensity versus wavelength is provided as an Origin Unicode Project file, which may be inspected with the Origin Viewer application.

Funders

I could be a scientist
PEF1\170015

Fellowship - Chirality in the 21st century: enantiomorphing chiral plasmonic meta/nano-materials
RGF\EA\180228

Science and Technology Facilities Council
https://doi.org/10.13039/501100000271

Look into my eyes
ST/R005842/1

Engineering and Physical Sciences Research Council
https://doi.org/10.13039/501100000266

EPSRC Centre for Doctoral Training in Condensed Matter Physics
EP/L015544/1

Publication details

Publication date: 10 May 2021
by: University of Bath

Version: 1

DOI: https://doi.org/10.15125/BATH-00989

URL for this record: https://researchdata.bath.ac.uk/id/eprint/989

Related papers and books

Murphy, A. W. A., Liu, Z., Gorbach, A. V., Ilie, A., and Valev, V. K., 2021. Doubly‐Resonant Enhancement of Second Harmonic Generation from a WS2 Nanomesh Polymorph with a Modified Energy Landscape. Laser & Photonics Reviews, 15(6), 2100117. Available from: https://doi.org/10.1002/lpor.202100117.

Contact information

Please contact the Research Data Service in the first instance for all matters concerning this item.

Contact person: Ventsislav Valev

Departments:

Faculty of Science
Physics

Research Centres & Institutes
Centre for Nanoscience and Nanotechnology
Centre for Photonics and Photonic Materials